The way the Black Keys do "Never Give You Up" reminds of of this badass underground Chicago soul tune from 1969 by this guy Renaldo Domino called "Not Too Cool To Cry".
Yes that is seriously the song title, and yes it is a dude singing (sounds a bit like a female).
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And if you dig it, check out this compilation (this song is on there) of amazing underground Chicago soul from the late 60's and early 70's...
http://www.numerogroup.com/catalog_detail.php?uid=00268